A nonlinear frequency shift caused by asymmetry of the coherent population trapping resonance: a generalization

We investigate the coherent population trapping resonance induced by a polychromatic optical field with an asymmetric spectrum, i.e., whose sidebands equidistant from the carrier have unequal powers. A situation is considered where a modulation is used to provide the so-called in-phase and quadrature signals in the optical field's transmission, which are used for stabilization of the local oscillator's frequency in chip-scale atomic clocks. In a general case, the frequencies of the signals nonlinearly depend on the optical field's intensity due to the asymmetry of the resonance. In this work, we demonstrate a) that this effect stems from a multi-peak structure of the resonance; b) a linear dependence of the frequency on the optical field's intensity at high modulation values; c) that the regime of the resolved structure has more advantages than suppression of the frequency shift due to the spectrum asymmetry.