Optica Open
Browse

Efficient extreme-ultraviolet high-order wave mixing from laser-dressed silica

Download (5.58 kB)
preprint
posted on 2023-01-10, 02:55 authored by Sylvianne D. C. Roscam Abbing, Filippo Campi, Brian de Keijzer, Corentin Morice, Zhuang-Yan Zhang, Maarten L. S. van der Geest, Peter M. Kraus
The emission of high-order harmonics from solids \cite{ghimire11a,schubert14a,luu15a,golde08a} under intense laser-pulse irradiation is revolutionizing our understanding of strong-field solid-light interactions \cite{ghimire11a,schubert14a,luu15a,vampa15b,yoshikawa17a,hafez18a,jurgens20a}, while simultaneously opening avenues towards novel, all-solid, coherent, short-wavelength table-top sources with tailored emission profiles and nanoscale light-field control\cite{franz19a,roscamCLEO21}. To date, broadband spectra have been generated well into the extreme-ultraviolet (XUV) \cite{luu15a,luu18b,han19a,uzan20a}, but the comparatively low conversion efficiency still lags behind gas-based high-harmonic generation (HHG) sources \cite{luu15a,luu18b}, and have hindered wider-spread applications. Here, we overcome the low conversion efficiency by two-color wave mixing. A quantum theory reveals that our experiments follow a novel generation mechanism where the conventional interband and intraband nonlinear dynamics are boosted by Floquet-Bloch dressed states, that make solid HHG in the XUV more efficient by at least one order of magnitude. Emission intensity scalings that follow perturbative optical wave mixing, combined with the angular separation of the emitted frequencies, make our approach a decisive step for all-solid coherent XUV sources and for studying light-engineered materials.

History

Disclaimer

This arXiv metadata record was not reviewed or approved by, nor does it necessarily express or reflect the policies or opinions of, arXiv.

Usage metrics

    Categories

    Licence

    Exports

    RefWorks
    BibTeX
    Ref. manager
    Endnote
    DataCite
    NLM
    DC