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Generation of Bright and Controllable Isolated Attosecond X-Ray Pulses from Synchronized Mid-Infrared and Ultra-short Ultraviolet Laser Fields

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posted on 2025-11-20, 17:01 authored by Davis Robinson, Kyle A. Hamer, Chelsea Kincaid, Michael Chini, Nicolas Douguet
We investigate, by solving the time-dependent Schrödinger equation in the single-active-electron approximation in helium, a two-color scheme for tabletop high-order harmonic generation (HHG) that combines a mid-infrared (MIR) driving field with an ultrashort ultraviolet (UV) pulse that could be generated via resonant dispersive wave emission in gas-filled hollow-core fibers. This configuration enables the generation of bright, isolated, and tunable attosecond X-ray pulses. In contrast to single-color driving schemes, which suffer from low conversion efficiency, unfavorable wavelength scaling, and limited spectral control, the MIR+UV approach provides a practical and controllable route for advancing tabletop ultrafast spectroscopy and real-time molecular imaging within current experimental capabilities.

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