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Generation of high-order harmonics with tunable photon energy and spectral width using double pulses

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posted on 2023-11-30, 19:37 authored by Lénárd Gulyás Oldal, Tamás Csizmadia, Peng Ye, Nandiga Gopalakrishna Harshitha, Amelle Zaïr, Subhendu Kahaly, Katalin Varjú, Miklós Füle, Balázs Major
This work theoretically investigates high-order harmonic generation in rare gas atoms driven by two temporally delayed ultrashort laser pulses. Apart from their temporal delay, the two pulses are identical. Using a single-atom model of the laser-matter interaction it is shown that the photon energy of the generated harmonics is controllable within the range of one eV -- a bandwidth comparable to the photon energy of the fundamental field -- by varying the time delay between the generating laser pulses. It is also demonstrated that high-order harmonics generated by double pulses have advantageous characteristics, which mimick certain properties of an extreme ultraviolet (XUV) monochromator. With the proposed method, a simpler setup at a much lower cost and comparatively higher spectral yield can be implemented in contrast to other approaches.

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