Overcoming Residual Timing Jitter in Pump-Probe Interferometry via Weak Value Amplification and Deep Learning

We introduce a hybrid methodology that synergistically combines weak value amplification (WVA) and deep learning to suppress the limiting effects of residual timing jitter in pump-probe interferometry, achieved through simulations of pump-induced time delays at a few-attosecond resolution. The WVA protocol, employing real weak values, amplifies the minute delay induced by sample perturbation, thereby translating it into a measurable shift of interference fringes. However, this amplification introduces significant fringe distortion. To address this, we deploy deep learning architectures as high-precision parameter estimators: a convolutional neural network regressor (CNN-Regressor) for direct delay estimation and a classifier (CNN-Classifier) for discrete delay categorization. These are systematically benchmarked against traditional Fourier-transform-based analysis. Two key conclusions are drawn: (i) The WVA technique consistently enhances measurement precision across all estimators by effectively increasing the signal-to-noise ratio (SNR). (ii) Both deep learning models surpass the traditional FFT approach; the CNN-Regressor achieves a higher SNR at small weak values, while the CNN-Classifier enables accurate estimation even under a challenging "$π$ phase shift" condition where conventional analysis fails. This synergistic combination of WVA and deep learning establishes a powerful framework for attosecond metrology, paving the way for enhanced precision in ultrafast spectroscopy.