Optical Fourier surfaces (OFSs), featuring sinusoidally profiled diffractive elements, manipulate light through patterned nanostructures and incident angle modulation. Compared to altering structural parameters, tuning elevation and azimuth angles offers greater design flexibility for light field control. However, angle-resolved responses of OFSs are often complex due to diverse mode excitations and couplings, complicating the alignment between simulations and practical fabrication. Here, we present a reality-infused deep learning framework, empowered by angle-resolved measurements, to enable real-time and accurate predictions of angular dispersion in quasi-OFSs. This approach captures critical features, including nanofabrication and measurement imperfections, which conventional simulation-based methods typically overlook. Our framework significantly accelerates the design process while achieving predictive performance highly consistent with experimental observations across broad angular and spectral ranges. Our study supports valuable insights into the development of OFS-based devices, and represents a paradigm shift from simulation-driven to reality-infused methods, paving the way for advancements in optical design applications.
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