Version 2 2023-06-08, 12:43Version 2 2023-06-08, 12:43
Version 1 2023-01-11, 22:18Version 1 2023-01-11, 22:18
preprint
posted on 2023-06-08, 12:43authored byHangyong Shan, Lukas Lackner, Bo Han, Evgeny Sedov, Christoph Rupprecht, Heiko Knopf, Falk Eilenberger, Johannes Beierlein, Nils Kunte, Martin Esmann, Kentaro Yumigeta, Kenji Watanabe, Takashi Taniguchi, Sebastian Klembt, Sven Höfling, Alexey V. Kavokin, Sefaattin Tongay, Christian Schneider, Carlos Antón-Solanas
The emergence of spatial and temporal coherence of light emitted from solid-state systems is a fundamental phenomenon, rooting in a plethora of microscopic processes. It is intrinsically aligned with the control of light-matter coupling, and canonical for laser oscillation. However, it also emerges in the superradiance of multiple, phase-locked emitters, and more recently, coherence and long-range order have been investigated in bosonic condensates of thermalized light, as well as in exciton-polaritons driven to a ground state via stimulated scattering. Here, we experimentally show that the interaction between photons in a Fabry-Perot microcavity and excitons in an atomically thin WSe$_2$ layer is sufficient such that the system enters the hybridized regime of strong light-matter coupling at ambient conditions. Via Michelson interferometry, we capture clear evidence of increased spatial and temporal coherence of the emitted light from the spatially confined system ground-state. The coherence build-up is accompanied by a threshold-like behaviour of the emitted light intensity, which is a fingerprint of a polariton laser effect. Valley-physics is manifested in the presence of an external magnetic field, which allows us to manipulate K and K' polaritons via the Valley-Zeeman-effect. Our findings are of high application relevance, as they confirm the possibility to use atomically thin crystals as simple and versatile components of coherent light-sources, and in valleytronic applications at room temperature.